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Abstract Rare-earth monopnictides are a family of materials simultaneously displaying complex magnetism, strong electronic correlation, and topological band structure. The recently discovered emergent arc-like surface states in these materials have been attributed to the multi-wave-vector antiferromagnetic order, yet the direct experimental evidence has been elusive. Here we report observation of non-collinear antiferromagnetic order with multiple modulations using spin-polarized scanning tunneling microscopy. Moreover, we discover a hidden spin-rotation transition of single-to-multiple modulations 2 K below the Néel temperature. The hidden transition coincides with the onset of the surface states splitting observed by our angle-resolved photoemission spectroscopy measurements. Single modulation gives rise to a band inversion with induced topological surface states in a local momentum region while the full Brillouin zone carries trivial topological indices, and multiple modulation further splits the surface bands via non-collinear spin tilting, as revealed by our calculations. The direct evidence of the non-collinear spin order in NdSb not only clarifies the mechanism of the emergent topological surface states, but also opens up a new paradigm of control and manipulation of band topology with magnetism.more » « less
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Huang, Zengle; Yi, Hemian; Min, Lujin; Mao, Zhiqiang; Chang, Cui-Zu; Wu, Weida (, Physical Review B)
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Yi, Hemian; Huang, Zengle; Shi, Wujun; Min, Lujin; Wu, Rui; Polley, C. M.; Zhang, Ruoxi; Zhao, Yi-Fan; Zhou, Ling-Jie; Adell, J.; et al (, Physical Review Research)
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